Integrating green chemistry principles into the fabrication of MIP electrochemical sensors for heavy metal monitoring

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dc.authorid0009-0008-2029-7899
dc.authorid0009-0007-3387-3202
dc.authorid0009-0009-3405-3905
dc.authorid0000-0001-6151-074X
dc.authorid0000-0001-5228-1682
dc.contributor.authorDorreh, Setareh
dc.contributor.authorKaya, Beril Sena
dc.contributor.authorAydemir, Zeynep
dc.contributor.authorAl Faysal, Abdullah
dc.contributor.authorGölcü, Ayşegül
dc.date.accessioned2026-06-26T05:56:09Z
dc.date.available2026-06-26T05:56:09Z
dc.date.issued2026
dc.departmentFakülteler, Eczacılık Fakültesi, Eczacılık Meslek Bilimleri Bölümü, Analitik Kimya Ana Bilim Dalı
dc.description.abstractHeavy metal contamination remains a critical global environmental issue due to the persistence, bioaccumulation, and toxicity of metal ions such as Pb2+, Cd2+, Hg2+, and As³+. Although conventional analytical techniques provide high sensitivity and accuracy, they often rely on energy-intensive instrumentation, hazardous reagents, and generate considerable chemical waste, raising concerns regarding their environmental sustainability. In this context, molecularly imprinted polymer (MIP)-based electrochemical sensors have emerged as promising alternatives, offering high selectivity, operational simplicity, and compatibility with miniaturized and in situ analysis. This review critically examines the integration of Green Analytical Chemistry (GAC) principles into the design and fabrication of MIP-based electrochemical sensors for heavy metal monitoring. Particular attention is given to material selection, polymerization strategies, template removal approaches, and electrode modification techniques, with emphasis on their environmental implications. The applicability of quantitative greenness assessment tools, including the Analytical Eco-Scale, GAPI, AGREE, and AGREEMIP, is discussed in the context of sensor development workflows, highlighting both their strengths and current limitations in addressing fabrication stages, nanomaterial synthesis, and end-of-life considerations. By identifying methodological bottlenecks, particularly solvent-intensive template removal and limited reusability, this review outlines practical directions for advancing more sustainable sensor platforms. Overall, the work provides a critical framework for aligning analytical performance with environmental responsibility in next-generation MIP-based electrochemical sensing systems.
dc.identifier.citationDorreh, S., Kaya, B. S., Aydemir, Z., Al Faysal, A., & Gölcü, A. (2026). Integrating green chemistry principles into the fabrication of MIP electrochemical sensors for heavy metal monitoring. Critical Reviews in Analytical Chemistry, pp. 1-19. https://doi.org/10.1080/10408347.2026.2684460
dc.identifier.doi10.1080/10408347.2026.2684460
dc.identifier.endpage19
dc.identifier.issn1040-8347
dc.identifier.issn1547-6510
dc.identifier.pmidPMID: 42324682
dc.identifier.scopusqualityQ1
dc.identifier.startpage1
dc.identifier.urihttps://doi.org/10.1080/10408347.2026.2684460
dc.identifier.urihttps://hdl.handle.net/20.500.13055/1520
dc.identifier.wosqualityQ1
dc.indekslendigikaynakWeb of Science
dc.indekslendigikaynakScopus
dc.indekslendigikaynakPubMed
dc.indekslendigikaynak.otherSCI-E - Science Citation Index Expanded
dc.institutionauthorKaya, Beril Sena
dc.institutionauthorid0009-0007-3387-3202
dc.language.isoen
dc.publisherTaylor & Francis
dc.relation.ispartofCritical Reviews in Analytical Chemistry
dc.relation.publicationcategoryDiğer
dc.rightsinfo:eu-repo/semantics/closedAccess
dc.subjectElectrochemical Sensors
dc.subjectGreen Analytical Chemistry (GAC)
dc.subjectHeavy Metal Detection
dc.subjectMolecularly Imprinted Polymers (MIPs)
dc.titleIntegrating green chemistry principles into the fabrication of MIP electrochemical sensors for heavy metal monitoring
dc.typeReview Article
dspace.entity.typePublication

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